Following the tremendous popular success of Jane Eyre, which earned her lifelong notoriety as a moral revolutionary, Charlotte Brontë vowed to write a sweeping social chronicle that focused on "something real and unromantic as Monday morning." Set in the industrializing England of the Napoleonic wars and Luddite revolts of 1811-12, Shirley (1849) is the story of two contrasting heroines. One is the shy Caroline Helstone, who is trapped in the oppressive atmosphere of a Yorkshire rectory and whose bare life symbolizes the plight of single women in the nineteenth century. The other is the vivacious Shirley Keeldar, who inherits a local estate and whose wealth liberates her from convention.

A work that combines social commentary with the more private preoccupations of Jane Eyre, Shirley demonstrates the full range of Brontë's literary talent. "Shirley is a revolutionary novel," wrote Brontë biographer Lyndall Gordon. "Shirley follows Jane Eyre as a new exemplar but so much a forerunner of the feminist of the later twentieth century that it is hard to believe in her actual existence in 1811-12. She is a theoretic possibility: what a woman might be if she combined independence and means of her own with intellect. Charlotte Brontë imagined a new form of power, equal to that of men, in a confident young woman [whose] extraordinary freedom has accustomed her to think for herself....Shirley [is] Brontë's most feminist novel."

The Professor was the first novel by Charlotte Brontë. It was written before Jane Eyre, but was rejected by many publishing houses. It was eventually published, posthumously, in 1857, with the approval of Charlotte Brontë's widower, Arthur Bell Nicholls, who took on the task of reviewing and editing the text.

With her final novel, Villette , Charlotte Brontë reached the height of her artistic power. First published in 1853, Villette is Brontë's most accomplished and deeply felt work, eclipsing even Jane Eyre in critical acclaim. Her narrator, the autobiographical Lucy Snowe, flees England and a tragic past to become an instructor in a French boarding school in the town of Villette. There she unexpectedly confronts her feelings of love and longing as she witnesses the fitful romance between Dr. John, a handsome young Englishman, and Ginerva Fanshawe, a beautiful coquette. The first pain brings others, and with them comes the heartache Lucy has tried so long to escape. Yet in spite of adversity and disappointment, Lucy Snowe survives to recount the unstinting vision of a turbulent life's journey - a journey that is one of the most insightful fictional studies of a woman's consciousness in English literature.